Picosecond near-to-mid-infrared absorption of pulse-injected small polarons in magnesium doped lithium niobate

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Freytag, F.; Booker, P.; Corradi, G.; Messerschmidt, S.; Krampf, A.; Imlau, M.: Picosecond near-to-mid-infrared absorption of pulse-injected small polarons in magnesium doped lithium niobate. In: Optical Materials Express 8 (2018), Nr. 6, S. 1505-1514. DOI: https://doi.org/10.1364/OME.8.001505

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Abstract: 
Femtosecond-pulse-induced (Epump = 2:5 eV) picosecond infrared absorption is studied in the spectral region between 0.30 eV and 1.05 eV in LiNbO3:Mg. We find a noninstantaneous mid-infrared absorption peak in the time domain up to 1 ps and a broad-band, long-lived absorption (maximum at 0.85 eV, width ≈ 0:5 eV), for t > 1 ps. The modelling succeeds by considering small Nb4+ Nb electron polaron formation along the sequence: (i) twophoton injection of hot electron-hole pairs at Nb-O-octahedra, (ii) dissociation and electron cooling by electron-phonon-scattering, and (iii) electron self-localization by strong electronphonon- coupling.
License of this version: OSA Open Access License
Document Type: Article
Publishing status: publishedVersion
Issue Date: 2018
Appears in Collections:An-Institute

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1 image of flag of Germany Germany 67 59.82%
2 image of flag of United States United States 24 21.43%
3 image of flag of China China 8 7.14%
4 image of flag of Russian Federation Russian Federation 4 3.57%
5 image of flag of Iran, Islamic Republic of Iran, Islamic Republic of 2 1.79%
6 image of flag of Indonesia Indonesia 2 1.79%
7 image of flag of No geo information available No geo information available 1 0.89%
8 image of flag of Mexico Mexico 1 0.89%
9 image of flag of France France 1 0.89%
10 image of flag of Spain Spain 1 0.89%
    other countries 1 0.89%

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