Carbon dioxide free production of hydrogen

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Stoppel, L.; Fehling, T.; Geißler, T.; Baake, E.; Wetzel, T.: Carbon dioxide free production of hydrogen. In: IOP Conference Series: Materials Science and Engineering 228 (2017), Nr. 1, No. 12016. DOI: https://doi.org/10.1088/1757-899X/228/1/012016

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Sum total of downloads: 678




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Abstract: 
The present report summarizes the theoretical modelling and experimental investigation results of the study on the direct thermal methane cracking. This work is a part of the LIMTECH-Project (Liquid Metal Technologies) funded of Helmholtz Alliance and was carried out from 2012 to 2017. The Project-part B5 "CO2-free production of hydrogen" focused on experimental testing and particularly on modelling the novel methane cracking method based on liquid metal technology. The new method uses a bubble column reactor, filled with liquid metal, where both the chemical reaction of methane decomposition and the separation of gas fraction from solid carbon occur. Such reactor system was designed and built in the liquid metal laboratory (KALLA) at KIT. The influences of liquid metal temperature distribution in reactor and feed gas flow rate on methane conversion ratio were investigated experimentally at the temperature range from 930 C to 1175 C and methane flow rate at the reactor inlet from 50 to 200 mLn/min. In parallel with experimental investigations, a thermochemical model, giving insight in the influence of the above mentioned parameters has been developed at KIT and a CFD model was developed at LUH to get an overview about the bubble dynamics in the reaction system. The influence of different bubble sizes and shapes, multi-inlet coalescence effects as well as the potential of electromagnetic stirring have been investigated.
License of this version: CC BY 3.0 Unported
Document Type: Article
Publishing status: publishedVersion
Issue Date: 2017
Appears in Collections:Fakultät für Elektrotechnik und Informatik

distribution of downloads over the selected time period:

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pos. country downloads
total perc.
1 image of flag of Germany Germany 517 76.25%
2 image of flag of United States United States 67 9.88%
3 image of flag of China China 13 1.92%
4 image of flag of No geo information available No geo information available 8 1.18%
5 image of flag of Russian Federation Russian Federation 7 1.03%
6 image of flag of Korea, Republic of Korea, Republic of 5 0.74%
7 image of flag of Indonesia Indonesia 5 0.74%
8 image of flag of Canada Canada 5 0.74%
9 image of flag of Netherlands Netherlands 4 0.59%
10 image of flag of Australia Australia 4 0.59%
    other countries 43 6.34%

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