Dynamics of valence-shell electrons and nuclei probed by strong-field holography and rescattering

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Walt, S.G.; Bhargava, Ram, N.; Atala, M.; Shvetsov-Shilovski, N.I. et al.: Dynamics of valence-shell electrons and nuclei probed by strong-field holography and rescattering. In: Nature Communications 8 (2017), 15651. DOI: https://doi.org/10.1038/ncomms15651

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Sum total of downloads: 240




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Abstract: 
Strong-field photoelectron holography and laser-induced electron diffraction (LIED) are two powerful emerging methods for probing the ultrafast dynamics of molecules. However, both of them have remained restricted to static systems and to nuclear dynamics induced by strong-field ionization. Here we extend these promising methods to image purely electronic valence-shell dynamics in molecules using photoelectron holography. In the same experiment, we use LIED and photoelectron holography simultaneously, to observe coupled electronic-rotational dynamics taking place on similar timescales. These results offer perspectives for imaging ultrafast dynamics of molecules on femtosecond to attosecond timescales.
License of this version: CC BY 4.0 Unported
Document Type: Article
Publishing status: publishedVersion
Issue Date: 2017
Appears in Collections:Fakultät für Mathematik und Physik

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pos. country downloads
total perc.
1 image of flag of Germany Germany 131 54.58%
2 image of flag of China China 64 26.67%
3 image of flag of United States United States 19 7.92%
4 image of flag of France France 8 3.33%
5 image of flag of Brazil Brazil 5 2.08%
6 image of flag of No geo information available No geo information available 3 1.25%
7 image of flag of Switzerland Switzerland 3 1.25%
8 image of flag of Portugal Portugal 1 0.42%
9 image of flag of Italy Italy 1 0.42%
10 image of flag of Hungary Hungary 1 0.42%
    other countries 4 1.67%

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