Asymmetry of Wigner's time delay in a small molecule

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Chacon, A.; Lein, M.; Ruiz, C.: Asymmetry of Wigner's time delay in a small molecule. In: Physical Review A - Atomic, Molecular, and Optical Physics 89 (2014), Nr. 5, 53427. DOI: https://doi.org/10.1103/PhysRevA.89.053427

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Sum total of downloads: 111




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Abstract: 
Ionization by an attosecond pulse launches an electron wave packet in the continuum which contains rich information about the pulse, the parent system, and the ionization dynamics. This emission process is not instantaneous in the sense that the electrons take a finite time to leave the potential. This time is closely related to the Wigner time. In this paper we introduce the stereo Wigner time delay, which measures the relative delay between electrons emitted to the left and right in an asymmetric system. We present a theoretical study of the delay in photoemission for a small asymmetric molecular system using the streaking technique. The stereo Wigner time delay shows advantages compared to previous schemes. Our numerical calculation shows that such a measurement removes the infrared laser-Coulomb coupling, which has been problematic in the interpretation of the measured delay in photoemission from atomic systems. © 2014 American Physical Society.
License of this version: Es gilt deutsches Urheberrecht. Das Dokument darf zum eigenen Gebrauch kostenfrei genutzt, aber nicht im Internet bereitgestellt oder an Außenstehende weitergegeben werden.
Document Type: Article
Publishing status: publishedVersion
Issue Date: 2014
Appears in Collections:Fakultät für Mathematik und Physik

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pos. country downloads
total perc.
1 image of flag of Germany Germany 56 50.45%
2 image of flag of United States United States 26 23.42%
3 image of flag of China China 11 9.91%
4 image of flag of Spain Spain 4 3.60%
5 image of flag of France France 3 2.70%
6 image of flag of Italy Italy 2 1.80%
7 image of flag of Iran, Islamic Republic of Iran, Islamic Republic of 2 1.80%
8 image of flag of Vietnam Vietnam 1 0.90%
9 image of flag of Japan Japan 1 0.90%
10 image of flag of Ireland Ireland 1 0.90%
    other countries 4 3.60%

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